Date of Award
6-2023
Document Type
Dissertation
Degree Name
Doctor of Philosophy (PhD)
Department
Department of Engineering Physics
First Advisor
Glen P. Perram, PhD
Abstract
The rubidium 5S-5D two-photon transitions were probed between 758-798 nm, where a six order of magnitude change in the cross section was observed and the polarization dependence was seen explicitly. Collisional rates are measured in cesium on the 6P-9S and 5D-10F transitions, with broadening rates as large as 710 MHz/Torr and shifting rates as large as 273 MHz/Torr. We observe Stark broadening on the cesium 5D-10F line shape, with Lorentzian width increasing from 200 MHz to 40 GHz. The influence of electron impact is discussed under these conditions and with 0-20 Torr of helium. Cascade amplified spontaneous emission is seen on the four cesium 8S-7P-7S transitions, with a maximum measured cw power of 32.4 mW. The mid-wave power and spatial profiles are examined as a function of pump power (up to 5.1 W), pump wavelength (detuned), and alkali density (1012 to 1014 cm-3).
AFIT Designator
AFIT-ENP-DS-23-J-016
Recommended Citation
True, Timothy M., "Non-degenerate Two-Photon Absorption and Excited State Line Shapes in Alkali Vapors" (2023). Theses and Dissertations. 7328.
https://scholar.afit.edu/etd/7328
Comments
A 12-month embargo was observed.
Approved for public release. PA case number on file.